By Mueller J.H.
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2 Biomimetic Complexation Studies. Pedersen [lJ found that macrocyc1ic polyethers, particularly those with the 18-crown-6 cavity, were capable of comp1exing ammonium ions. Cram [6J pointed out that the addition of extra units could give such compounds more shape and additional binding sites. Since then a number of researchers have prepared host molecules which contain a combination of shaped and charged side units in efforts to duplicate the chiral and electrostatic recognition of guest molecules afforded in natural systems by enzymes and proteins.