By Stefan Kubik (auth.), Markus Albrecht, Ekkehardt Hahn (eds.)
Molecular Cages and drugs with Functionalized internal Surfaces, by means of Stefan Kubik. Drug supply by way of Water-Soluble Organ metal Cages, by means of Bruno Therrien. Reversibly accelerated Encapsulation Complexes, by means of Dariush Ajami und Julius Rebek. box Molecules in accordance with Imine kind Ligands, through A. Carina Schulze und Iris M. Oppel. Molecular drugs Derived from Resorcinarenes via Metal-Coordination, through Tobias Schröder, Satya Narayan Sahu und Jochen Mattay. Coronates, round bins, Bowl-Shaped Surfaces, Porous 1D-, 2D-, 3D-Metallo-Coordination Polymers, and Metallodendrimers, through Rolf W. Saalfrank und Andreas Scheurer.
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References . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . . 36 37 39 42 44 48 52 52 B. Therrien (*) Institut de chimie, Universite´ de Neuchaˆtel, Av. ch 36 B. Therrien Abbreviations bipy bpe bpp bpy Cp Cp* DAniF dcbq dhbq doaq donq dotq en phen tpp tppp tpt 4,40 -Bipyridine 1,2-Bis(4-pyridyl)ethylene 5,15-Bis(4-pyridyl)-10,20-diphenylporphyrin 2,20 -Bipyrimidine Cyclopentadienyl Pentamethylcyclopentadienyl N,N0 -Di(p-anisyl)formamidinate 2,5-Dichloro-1,4-benzoquinone-3,6-diolato 1,4-Benzoquinone-2,5-diolato 1,4-Anthraquinone-9,10-diolato 1,4-Naphthoquinone-5,8-diolato Tetracene-5,12-dione-6,11-diolato Ethylenediamine 4,7-Phenanthroline 5,10,15,20-Tetra(4-pyridyl)porphyrin 5,10,15-Tris(4-pyridyl)-20-phenylporphyrin 1,3,5-Tris(4-pyridyl)triazine 1 Introduction The design of molecular hosts to encapsulate guest molecules in a confined environment is receiving considerable attention due to the analogy of these systems with the mode of action of enzymes.
These examples illustrate the versatility of half-sandwich complexes in the construction of two- and three-dimensional assemblies, thus providing a multitude of possibilities for producing new metalla-hosts for various applications. 5 Organometallic Assemblies Composed of Half-Sandwich Complexes for Biological Applications Most macrocycles composed of half-sandwich complexes are positively charged and water soluble. The water solubility and stability of organometallic compounds are advantageous, and organometallic chemistry in aqueous-phase is growing rapidly .
In addition, directionality of the interactions inside the receptor cavity induces an ordered arrangement of the included guest molecules, an effect that is probably not so important for smaller receptors where steric effects are usually sufficient to restrict the motion of the guests. In larger cavities, however, translational motions of the guests are often less difficult and an ordered arrangement of guest molecules can only be achieved when the guest finds positions on the inner cavity surface to which it can bind.